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Doing a search for CO2 in the IO Reference it looks like the user can specify the concentration with these objects:

ZoneAirContaminantBalance

ZoneContaminantSourceAndSink:CarbonDioxide

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No.2 Revision

Doing a search for CO2 in the 8.1 IO Reference it looks like the user can specify the concentration with these objects:

ZoneAirContaminantBalance

ZoneContaminantSourceAndSink:CarbonDioxide